Download e-book for iPad: Advances in Chemical Physics, Volume 148 by Stuart A. Rice, Aaron R. Dinner

By Stuart A. Rice, Aaron R. Dinner

ISBN-10: 1118122356

ISBN-13: 9781118122358

ISBN-10: 1118158717

ISBN-13: 9781118158715

The Advances in Chemical Physics series—the leading edge of analysis in chemical physics

The Advances in Chemical Physics sequence presents the chemical physics and actual chemistry fields with a discussion board for serious, authoritative reviews of advances in each region of the self-discipline. packed with state-of-the-art study stated in a cohesive demeanour now not stumbled on in other places within the literature, each one quantity of the Advances in Chemical Physics sequence deals contributions from the world over well known chemists and serves because the ideal complement to any complex graduate type dedicated to the research of chemical physics.

This quantity explores:

  • keep an eye on of Quantum Phenomena (Constantin Brif, Raj Chakrabarti, and Herschel Rabitz)

  • Crowded fees in Ion Channels (Bob Eisenberg)

  • Colloidal Crystallization among and 3 Dimensions (H. Lowen, E.C. Oguz, L. Assoud, and R. Messina)

  • Statistical Mechanics of beverages and Fluids in Curved area (Gilles Tarjus, FranCois Sausset, and Pascal Viot)

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Extra resources for Advances in Chemical Physics, Volume 148

Example text

The pulse was shaped prior to propagation through the fiber, and AFC maximized the fluorescence signal contrast between two fluorescent proteins. A novel phase modulation technique for ultrabroadband laser pulses was developed for selective excitation of multiple fluorophores in TPEF microscopy [524]. This technique was applied to dual-color imaging of cells containing two types of fluorescent proteins, and AFC was employed to find the phase modulation that maximizes or minimizes the individual TPEF intensity from one of the fluorophores.

However, it was argued [509, 510] that in nonimpulsive SRS, the relative peak heights in the Raman spectrum do not reflect the relative populations of the vibrational modes and that control of the spectral features demonstrated in the experiments [505–508] does not involve quantum interference of vibrational excitations, but rather is based on classical nonlinear optical effects. Another important area of nonlinear molecular spectroscopy is control of molecular vibrational modes via coherent anti-Stokes Raman scattering (CARS).

In 2001, Levis and coworkers [483] used AFC with shaped, strong-field laser pulses to demonstrate highly selective cleavage of chemical bonds in polyatomic organic molecules in the gas phase. The use of strong laser fields (with intensities of about 1013 W cm−2 ) helps to effectively increase the available bandwidth, as transitions to excited molecular states are facilitated by the dynamic Stark shift. This effect opens up many reaction pathways that are inaccessible in the weak-field (perturbative) regime due to resonant spectral restrictions [12].

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Advances in Chemical Physics, Volume 148 by Stuart A. Rice, Aaron R. Dinner


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